Partial Synthesis of Novel Ligands for the Catalytic Activation of Hydrogen Peroxide in Pursuit of Green Oxidative Chemistry

Author

Daniel Kaplan

Date of Award

2008

Document Type

Thesis

Degree Name

Bachelors

Department

Natural Sciences

First Advisor

Scudder, Paul

Keywords

Catalytic Activation, Hydrogen Peroxide, Green Chemistry

Area of Concentration

Chemistry

Abstract

Green chemistry, at its core, is about developing a chemically sustainable society. Water borne pollution is a growing concern throughout the world. As nations develop technologically, the potential for rapidly increasing pollution becomes a growing issue. A safe, clean, and reusable method for treating water must be developed. Hydrogen peroxide when catalytically activated by complexed high valent iron provides a powerful tool for treating and eliminating water borne pollution. Based off the natural model of cytochrome P450, an increasing number of synthetic ligands have been developed. This thesis details the development and partial synthesis of a novel ligand, designed to stabilize high valent iron for the catalytic activation of hydrogen peroxide. The final goal of this thesis is the physical attachment of the ligand for simplified extraction and reuse. A synthetic scheme was planned and then modified as necessary, when complications in synthesis arose. All but the final step of the synthesis was completed.

Rights

This bibliographic record is available under the Creative Commons CC0 public domain dedication. The New College of Florida, as creator of this bibliographic record, has waived all rights to it worldwide under copyright law, including all related and neighboring rights, to the extent allowed by law.

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